期刊
ADVANCED FUNCTIONAL MATERIALS
卷 27, 期 3, 页码 -出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/adfm.201603921
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资金
- National Research Foundation (NRF) - Ministry of Science, ICT and Future Planning [NRF-2013R1A1A2074550, NRF-2016R1A4A1010735]
- Korea Science and Engineering Foundation (KOSEF) - Korean Government (MEST) [NRF-2015M1A2A2056557]
- C1 Gas Refinery Program through the NRF - Ministry of Science, ICT and Future Planning [NRF-2015M3D3A1A01065440]
- National Research Foundation of Korea [2016R1A4A1010735, PAL-2017, 2015M1A2A2056555, 2013R1A1A2074550, 2015M3D3A1A01064957] Funding Source: Korea Institute of Science & Technology Information (KISTI), National Science & Technology Information Service (NTIS)
A general method to synthesize mesoporous metal oxide@ N-doped macroporous graphene composite by heat-treatment of electrostatically co-assembled amine-functionalized mesoporous silica/metal oxide composite and graphene oxide, and subsequent silica removal to produce mesoporous metal oxide and N-doped macroporous graphene simultaneously is reported. Four mesoporous metal oxides (WO3-x, Co3O4, Mn2O3, and Fe3O4) are encapsulated in N-doped macroporous graphene. Used as an anode material for sodium-ion hybrid supercapacitors (Na-HSCs), mesoporous reduced tungsten oxide@ N-doped macroporous graphene (m-WO3-x@ NM-rGO) gives outstanding rate capability and stable cycle life. Ex situ analyses suggest that the electrochemical reaction mechanism of m-WO3-x@ NM-rGO is based on Na+ intercalation/de-intercalation. To the best of knowledge, this is the first report on Na+ intercalation/de-intercalation properties of WO3-x and its application to Na-HSCs.
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