期刊
SCIENCE ADVANCES
卷 5, 期 1, 页码 -出版社
AMER ASSOC ADVANCEMENT SCIENCE
DOI: 10.1126/sciadv.aau0582
关键词
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资金
- National Natural Science Foundation of China [21688102, 21733006, 21590802]
- National Key Research and Development Program of China [2017YFA0206500]
- NSF [CHE-1566636]
- U.S. Department of Energy Office of Science, Office of Basic Energy Sciences [DE-SC0010616, DE-SC0015997]
First-principles treatments of quantum molecular reaction dynamics have reached the level of quantitative accuracy even in cases with strong non-Born-Oppenheimer effects. This achievement permits the interpretation of puzzling experimental phenomena related to dynamics governed by multiple coupled potential energy surfaces. We present a combined experimental and theoretical study of the photodissociation of formyl radical (HCO). Oscillations observed in the distribution of product states are found to arise from the interference of matter waves-a manifestation analogous to Young's double-slit experiment.
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