期刊
ACS ENERGY LETTERS
卷 4, 期 1, 页码 192-202出版社
AMER CHEMICAL SOC
DOI: 10.1021/acsenergylett.8b01833
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资金
- Department of Science and Technology, New Delhi, India
- UKRI Global Challenge Research Fund project, SUNRISE [EP/P032591/1]
- Engineering and Physical Sciences Research Council, U.K. [EP/M025330/1]
- EPSRC [EP/P032591/1] Funding Source: UKRI
The process of carrier multiplication via singlet fission can potentially exceed the Shockley-Queisser limit on the efficiency of single-junction photovoltaics. In the recent past, theoretical analysis provided the principal guidelines on molecular design strategies for singlet fission. In this Perspective, we focus instead on correlating experimental results for different classes of reported singlet fission materials to identify principles to aid in the design of new molecules for efficient intramolecular singlet fission. Building on an evaluation of several series of multichromophoric and polymeric singlet fission materials, we extract new suggested strategies for molecular design.
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