期刊
MATERIALS
卷 12, 期 2, 页码 -出版社
MDPI
DOI: 10.3390/ma12020276
关键词
design and fabrication strategy; ordered mesoporous metal oxides; heterogeneous catalyst; carbon dioxide; catalytic conversion
类别
资金
- National Natural Science Foundation of China [21503113, 21577065, 21503142, 91543115]
- International ST Cooperation Program of China [2014DFA90780]
- Environmental protection projects of Jiangsu province [2017022]
- Priority Academic Program Development of Jiangsu Higher Education Institutions
- Startup Foundation of Nanjing University of Information Science and Technology
In the past two decades, great progress has been made in the aspects of fabrication and application of ordered mesoporous metal oxides. Ordered mesoporous metal oxides have attracted more and more attention due to their large surface areas and pore volumes, unblocked pore structure, and good thermal stabilities. Compared with non-porous metal oxides, the most prominent feature is their ability to interact with molecules not only on their outer surface but also on the large internal surfaces of the material, providing more accessible active sites for the reactants. This review carefully describes the characteristics, classification and synthesis of ordered mesoporous metal oxides in detail. Besides, it also summarizes the catalytic application of ordered mesoporous metal oxides in the field of carbon dioxide conversion and resource utilization, which provides prospective viewpoints to reduce the emission of greenhouse gas and the inhibition of global warming. Although the scope of current review is mainly limited to the ordered mesoporous metal oxides and their application in the field of CO2 catalytic conversion via heterogeneous catalysis processes, we believe that it will provide new insights and viewpoints to the further development of heterogeneous catalytic materials.
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