期刊
ACS CATALYSIS
卷 9, 期 3, 页码 2063-2067出版社
AMER CHEMICAL SOC
DOI: 10.1021/acscatal.8b04351
关键词
electrochemistry; C-C activation; amination; oxidation; rearrangements
资金
- National Natural Science Foundation of China [21632001, 81821004, 21772002]
- National Basic Research Program of China (973 Program) [2015CB856600]
- Drug Innovation Major Project [2018ZX09711-001]
In contrast to the recent breakthrough in electrochemical C-H aminations, the electrochemically oxidative C-N bond formation through a C-C bond cleavage is rarely studied. This work describes an electrochemical C-C amination of alkylarenes for the efficient synthesis of versatile anilines, as well as carbonyl compounds. With the cheap and durable graphite plates as electrodes, and in a simple undivided cell, this protocol is much more economical with the consumption of electricity.
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