期刊
SYNTHESIS-STUTTGART
卷 50, 期 24, 页码 4715-4745出版社
GEORG THIEME VERLAG KG
DOI: 10.1055/s-0037-1610297
关键词
high-valent metal complexes; flavins; biomimetics; C-H oxidations; sustainable oxidations; green oxidations
资金
- project 'OPENSCREEN-GR' under the Action 'Reinforcement of the Research and Innovation Infrastructure' - Operational Program 'Competitiveness, Entrepreneurship and Innovation' (NSRF 2014-2020) [MIS 5002691]
- Greece and the European Union (European Regional Development Fund)
Monooxygenases are not only some of the most versatile machineries in our lives, but also some of the most explored enzymes in modern organic synthesis. They provide knowledge and inspiration on how the most abandoned oxidant, dioxygen, can be activated and utilized to deliver selective oxidations. This review presents an outline in the mechanisms that Nature uses to succeed in these processes and recent indicative examples on how chemists use this knowledge to develop selective oxidation protocols based on dioxygen as the terminal oxidant.
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