期刊
SYNTHESIS-STUTTGART
卷 50, 期 23, 页码 4501-4524出版社
GEORG THIEME VERLAG KG
DOI: 10.1055/s-0037-1610284
关键词
azomethine imines; alkynes; cycloadditions; click chemistry; pyrazolines
资金
- Slovenian Research Agency (ARRS) [P1-0179]
Although the first example of copper-catalyzed azomethine imine-alkyne cycloaddition (CuAIAC) was published only a year after the seminal papers of Meldal and Sharpless on Cu-catalyzed azidealkyne cycloaddition (CuAAC), the CuAIAC reaction has remained overlooked by the synthetic community for almost a decade. Since 2010, however, CuAIAC reaction started to emerge as a promising supplement to the well-known CuAAC reaction. The present review surveys primarily the literature on CuAIAC reaction since 2003. Beside this, azomethine imine-alkyne cycloadditions catalyzed by other metals, selected examples of metal-free reactions, and related [3+ 3] and [3+ 4] cycloadditions of azomethine imines are presented. All these experimental data indicate the viability of CuAIAC in organic synthesis and the applicability in 'click' chemistry.
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