期刊
PHYSICA STATUS SOLIDI A-APPLICATIONS AND MATERIALS SCIENCE
卷 216, 期 3, 页码 -出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/pssa.201800522
关键词
gadolinium; ion implantation; optical absorption; quasi-dynamic disorder; silica
资金
- Ministry of Education and Science of the Russian Federation [3.1485.2017/4.6]
- Act 211 Government of the Russian Federation [A03.21.0006]
The electronic structure and optical properties of silica glass implanted with Gd-ions by the pulsed implantation technique are studied. Experimental XPS data combined with the theoretical density functional theory (DFT)-modeling establish the most probable scenarios for Gd-embedding at the interstitial and substitutional positions in silica before and after thermal annealing. The optical absorption spectra are analyzed within two spectral regions of direct interband transitions and exponential Urbach tails. The influence of both radiation and thermal treatment on the overall structural disorder of host-matrix is determined using fundamental optical parameters (band gap, phonon energy). The local atomic displacements caused by the implantation damage and thermal recovery of host-structure for as-implanted and annealed samples are quantitatively estimated.
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