期刊
ORGANIC LETTERS
卷 20, 期 23, 页码 7731-7734出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.8b03518
关键词
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资金
- NSFC [21672169]
- Key Science and Technology Innovation Team of Shaanxi [2017KCT-37]
- Key Laboratory Project of Xi'an [201805058ZD9CG42]
A highly chemoselective intermolecular annulation reaction of phenol-based biaryls with bromoalkyl alkynes has been successfully developed by palladium/norbornene catalysis. This domino process was accomplished by following a cascade of Catellani-type C-H functionalization, alkyne migratory insertion, and arene dearomatization, thus leading to a large number of spiro[4,5]decane-embedded polycyclic molecules bearing various functional groups in moderate to excellent yields.
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