期刊
ORGANIC LETTERS
卷 21, 期 3, 页码 618-622出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.8b03652
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资金
- National Natural Science Foundation of China [21773273, 21473226]
- Key Research Program of Frontier Sciences, CAS [QYZDJ-SSW-SLH051]
- Natural Science Foundation of Jiangsu Province [BK20170420]
A highly efficient strategy for the enantioselective oxidation of methylene C-H of spirocyclic oxindoles and dihydroquinolinones has been established, in which an earth-abundant manganese catalyst and hydrogen peroxide are used. Noteworthy, the manganese catalyst can be applied to the asymmetric hydroxylation of spirocyclic 2,3-dihydroquinolin-4-ones with 94-99% ee.
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