期刊
ACS NANO
卷 10, 期 6, 页码 5730-5739出版社
AMER CHEMICAL SOC
DOI: 10.1021/acsnano.5b07355
关键词
thermoelectric; tin selenide; nanosheet; exfoliation; poly(3,4-ethylenedioxythiophene):poly(styrenesulfonate)
类别
资金
- NRF - MEST [2014R1A2A1A11049625]
- National Research Foundation of Korea [2014R1A2A1A11049625] Funding Source: Korea Institute of Science & Technology Information (KISTI), National Science & Technology Information Service (NTIS)
Tin selenide (SnSe) nanosheets (NSs) are prepared by hydrothermal lithium-intercalation and a subsequent exfoliation process from a SnSe ingot. Conducting polymer poly(3,4-ethylenedioxythiohene):poly(styrenesulfonate) (PEDOT:PSS)-based thermoelectric composites are fabricated with varying SnSe NSs content, and the thermoelectric properties of the composites are examined at 300 K. The exfoliated SnSe particles show thin two-dimensional sheet-like structures that are evenly distributed into the PEDOT:PSS matrix. The significantly enhanced power factor (S-2.sigma of the SnSe NS/PEDOT:PSS composites with increasing SnSe NSs content can be explained by the potential difference at the interface between the SnSe and PEDOT:PSS. The fabricated SnSe NS/PEDOT:PSS composites show a maximum figure of merit (ZT) of 0.32 at a SnSe NSs loading of 20 wt %. The mixing of inorganic nanoparticles with the conducting polymer matrix forms products with extremely low thermal conductivities, which is a promising strategy for the realization of polymer based efficient thermoelectric applications.
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