Megafilament in air formed by self-guided terawatt long-wavelength infrared laser

The diffraction-compensated propagation of high-power laser beams in air could open up new opportunities for atmospheric applications such as remote stand-off detection, long-range projection of high-energy laser pulses and free-space communications. Here, we experimentally demonstrate that a self-guided terawatt picosecond CO2 laser beam forms in air a single centimetre-scale-diameter megafilament that, in comparison with a short-wavelength laser filament, has four orders of magnitude larger cross-section and guides many joules of pulse energy over multiple Rayleigh distances at a clamped intensity of similar to 10(12) W cm(-2). We discover that this megafilament arises from the balance between self- focusing, diffraction and defocusing caused by free carriers generated via many-body Coulomb-induced ionization that effectively decrease the molecular polarizability during the long-wavelength laser pulse. Modelling reveals that this guiding scheme may enable transport of high-power picosecond infrared pulses over many kilometres in the 8-14 mu m atmospheric transmission window.