4.8 Article

Vapor Growth and Tunable Lasing of Band Gap Engineered Cesium Lead Halide Perovskite Micro/Nanorods with Triangular Cross Section

期刊

ACS NANO
卷 11, 期 2, 页码 1189-1195

出版社

AMER CHEMICAL SOC
DOI: 10.1021/acsnano.6b07374

关键词

cesium lead halide perovskites; triangular micro/nanorods; tunable lasers; vapor-phase growth

资金

  1. National Natural Science Foundation of China [51302077, 51525202, 61574054, 11374092]
  2. Hunan Provincial Natural Science Foundation of China [2015JJ3049]
  3. Fundamental Research Funds for the Central Universities

向作者/读者索取更多资源

Although great efforts have been devoted to the synthesis of halide perovskites nanostructures, vapor growth of high-quality one-dimensional cesium lead halide nanostructures for tunable nanoscale lasers is still a challenge. Here, we report the growth of high-quality all-inorganic cesium lead halide alloy perovskite micro/nanorods with complete composition tuning by vapor-phase deposition. The as-grown micro/nanorods are single-crystalline with a triangular cross section and show strong photoluminescence which can be tuned from 415 to 673 urn by varying the halide composition. Furthermore, these single-crystalline perovskite micro/nanorods themselves function as effective Fabry-Perot cavities for nanoscale lasers. We have realized room temperature tunable lasing of cesium lead halide perovskite with low lasing thresholds (similar to 14.1 mu J cm(-2)) and high Q factors (similar to 3500).

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