期刊
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
卷 140, 期 50, 页码 17369-17373出版社
AMER CHEMICAL SOC
DOI: 10.1021/jacs.8b10888
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资金
- DOE Office of Science Graduate Student Research (SCGSR) program
- National Science Foundation [CHE-1562140, CHE-1800584]
- DOE Office of Science through the Heavy Element Chemistry program for X-ray crystallography and spectroscopy at LANL
Reduction of IU(NHAriPr6)(2) (Ar-iPr6 = 2,6-(2,4,6-(Pr3C6H2)-Pr-i)(2)C6H3) results in a rare example of a U(II) complex, U(NHAriPr6)(2), and the first example that is a neutral species. Here, we show spectroscopic and magnetic studies that suggest a 5f(4)6d(0) valence electronic configuration for uranium, along with characterization of related U(III) complexes.
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