期刊
JOURNAL OF ORGANIC CHEMISTRY
卷 83, 期 21, 页码 13587-13594出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.joc.8b02249
关键词
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资金
- MEXT [17H06091]
The alkylation of C-H bonds with N-vinylphthalimide by a rhodium-catalyzed reaction of aromatic amides containing an 8-aminoquinoline moiety as the directing group is reported. N-Vinylphthalimide functions as a 2-aminoethylating reagent. The resulting alkylated products can be converted into 3,4-dihydroisoquinolin-1(2H)-one derivatives in a one-pot transformation. Deuterium-labeling experiments suggest that the reaction proceeds through a carbene mechanism.
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