期刊
ENERGIES
卷 11, 期 11, 页码 -出版社
MDPI
DOI: 10.3390/en11112948
关键词
silicon; pressure; full cell; cycle aging; calendar aging; temperature influence; DoD influence; C-rate influence
资金
- European Union's Horizon 2020 research and innovation program [653531]
In this research, twenty-four high capacity (1360 mAh) NMC622/Si-alloy Li-ion full pouch cells with high silicon-alloy content (55%) are cycle aged under seven different cycling conditions to study the effect of different stressors on the cycle life of Si-anode full cells, among which are the effect of ambient temperature, Depth of Discharge (DoD) and the discharge current. The cells are volumetrically constrained at an optimal initial pressure to improve their cycle life, energy and power capabilities. Furthermore, the innovative test setup allows measuring the developed pressure as a result of repeated (de-)lithiation during battery cycling. This uniquely vast testing campaign on Si-anode full cells allows us to study and quantify independently the influence of different stress factors on their cycle life for the first time, as well as to develop a new capacity fade model based on an observed linear relationship between capacity retention and total discharge capacity throughput.
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