期刊
ELECTROCHIMICA ACTA
卷 293, 期 -, 页码 419-425出版社
PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/j.electacta.2018.10.059
关键词
Co9S8; Graphene; Supercapacitor; Composites
资金
- National Natural Science Foundation of China (NSFC) [21501152, 21571159, 21441003]
- Program for Changjiang Scholars and Innovative Research Team in University [IRT15R61]
- Foundation of Zhengzhou University of Light Industry Projects for Public Entrepreneurship [2014BSJJ054]
- Province Science and Technology Open Cooperation Project [172106000065]
- Public Innovation of ZZULI [CLY20170165, 2017ZCKJ215]
- Key Program of Henan Province for Science and Technology [CLY20180110, 162102210212]
Island-like Co9S8 nanoparticles composed of two-dimensional (2D) Co9S8 nanosheets in-situ grew and were dispersed evenly on the surface of 2D N-doping graphene (NGR), which produced the Co9S8@NGR nanocomposites using a simple solvothermal method. In this solvothermal process, graphene oxides were reduced and doped with nitrogen (N) simultaneously. The Co9S8@NGR nanocomposites delivered an ultra-high specific capacitance of 2992 Fg(-1) in a potential window of 0.5 Vat 1 A g(-1). Moreover, an asymmetric supercapacitor (ASC) constructed by Co9S8@NGR as the positive electrode and by activated carbon (AC) as the negative electrode showed the density of 88.81 W h kg(-1) at a power density of 0.63 kW kg(-1), the power density of 21.80 kW kg(-1) at the energy density of 30.30 W h kg(-1), and the favorable cycle stability with 80.61% specific capacity retention at a current density of 10 A g(-1) after 10000 cycles. (C) 2018 Elsevier Ltd. All rights reserved.
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