期刊
CHEMCATCHEM
卷 11, 期 2, 页码 724-728出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/cctc.201801626
关键词
Fe-based catalyst; N-doped porous carbon; Chemoselectivity; Nitro compounds
资金
- National Natural Science Foundation of China [NSFC: 21401004, 21201062]
- Natural Science Foundation of Anhui Province [1508085QB36]
- Doctoral Scientic Research Foundation [070138]
Herein, we designed and prepared a novel Fe/Fe2O3-based catalyst, in which a remarkable synergistic effect has been revealed between Fe and Fe2O3 encapsulated in N-doping porous carbon. The Fe-based catalysts were fabricated via pyrolysis a mixture of MIL-101(Fe) and melamine. The catalyst exhibits exceptionally high catalytic activity (TOFs up to 8898 h(-1) which is about 100 times higher than the similar kinds of catalysts) and chemoselectivity for nitroarene reduction under mild conditions.
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