期刊
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
卷 58, 期 5, 页码 1355-1360出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/anie.201811032
关键词
cyclization; fluorination; phosphine oxide; superacid; superelectrophile
资金
- Universite de Poitiers
- CNRS
- Region Nouvelle Aquitaine
- Ludwig-Maximilian University Munich (LMU)
- F-Select GmbH
- French Fluorine Network
- Labex SynOrg [ANR-11-LABX-0029]
- Normandie Universite
Unambiguously confirmed by low-temperature in situ NMR experiments, X-ray diffraction and vibrational spectroscopy, phosphonium-carbenium superelectrophiles are shown to be generated in strong acidic conditions. Representing crucial intermediates, their exploitation allows for the synthesis of unprecedented fluorinated (cyclic) phosphine oxides.
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