期刊
ADVANCED SYNTHESIS & CATALYSIS
卷 361, 期 6, 页码 1307-1312出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/adsc.201801346
关键词
Dual catalysis; pi-Allyl palladium complex; Rhodium-carbenoids; Quaternary carbon center; Oxindoles
资金
- National Natural Science Foundation of China [21402154, 21502150]
- Chinese Universities Scientific Fund [2452016093]
- Youth Training Project of Northwest AF University [2452017034, 2452016006]
A chemo-selective Rh(II)/Pd(0) dual catalysis that promotes one-pot synthesis of C3-quaternary allylic oxindoles from N-aryl-alpha-diazo-beta-ketoamides and functionalized allyl carbonates in good to excellent yields has been developed. The efficiency of this transformation relies on the choice of Rh(II)/Pd(0) dual catalysis strategy that enabled cascade intramolecular aryl C-H insertion and allylic alkylation under mild conditions.
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