期刊
JOURNAL OF MATERIALS CHEMISTRY C
卷 2, 期 14, 页码 2622-2634出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c3tc31933d
关键词
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资金
- National Research Foundation of Korea (NRF) grant
- Korea government (MEST) [2012R1A2A2A01015654]
- Converging Research Center Program through the Ministry of Science, ICT and Future Planning, Korea [2013K000162]
- Basic Science Research Program through the National Research Foundation of Korea (NRF) Grant
- Korea Government (MSIP) [NRF-2010-0027963]
- Chungcheong institute for regional program evaluation promotion project of the Korean Ministry of Knowledge Economy [R0001445]
- Kwangwoon University
- Korea Evaluation Institute of Industrial Technology (KEIT) [R0001445] Funding Source: Korea Institute of Science & Technology Information (KISTI), National Science & Technology Information Service (NTIS)
- National Research Foundation of Korea [2012R1A2A2A01015654] Funding Source: Korea Institute of Science & Technology Information (KISTI), National Science & Technology Information Service (NTIS)
We herein report an investigation of graphene oxide (GO) thin layers fabricated by simple horizontal-dip (H-dip) coating on an indium-tin-oxide (ITO) anode as used in solution-processable organic semiconducting devices. Homogeneous and smooth GO thin films were successfully deposited via an aqueous dispersion of GO on an ITO electrode, with a high surface coverage and low surface roughness, and a thickness controlled by H-dip coating. The use of an H-dip-coated GO film as a hole-injecting interfacial layer (IFL) in organic light-emitting diodes (OLEDs) resulted in a remarkable improvement in device performance (17 cd A(-1)), better than that (12 cd A(-1)) of a reference OLED with a spin-coated GO IFL. Stacked bi-IFLs of GO/poly(ethylenedioxythiophene):poly(styrene sulfonate) (GO/PEDOT:PSS) fabricated by H-dip coating were also investigated as hole-injecting IFLs in OLEDs, and these showed an even better device performance (23 cd A(-1)). Furthermore, it was also shown that polymer solar cells with H-dip-coated GO/PEDOT:PSS hole-collecting bi-IFLs exhibited a remarkable improvement in power conversion efficiency (6.9%), which was also higher than that (4.8%) obtained with spin-coated bi-IFLs. These results clearly indicate that the H-dip-coating of GO(/PEDOT:PSS) can effectively modify the ITO interface to yield efficient hole-selective IFLs, representing considerable promise for use as an alternative to spin-coated IFLs in the mass production of solution-processable organic semiconducting devices.
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