期刊
JOURNAL OF MATERIALS CHEMISTRY A
卷 2, 期 23, 页码 8660-8667出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c4ta00860j
关键词
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资金
- National Science and Technology Major Project [2011ZX02707, 2012CB825800, 2013CB932702]
- National Natural Science Foundation of China [11104303, 11274333, 11204339, 61136005, 51132006]
- Chinese Academy of Sciences [KGZD-EW-303, XDA02040000, XDB04010500, XDB01010200, Y321311401]
- Suzhou Planning Project of Science and Technology [ZXG2012028]
Carbon quantum dots (CQDs) have been intensively investigated due to their interesting electrochemical and photoluminescent properties. Here, we report a novel method for large-scale preparation of heavy doped CQDs with tunable photoluminescence. In the present synthetic process, the carbon nanoparticles from Chinese ink were oxidized and cut simultaneously using a mature process to obtain oxidized-CQDs as precursors, and then the heteroatom (N, S or Se) doped CQDs were obtained by a one-step hydrothermal reduction and in situ doping treatment. The heavy doped CQDs are just 1-6 nm size, and have improved photoluminescence with different emission wavelengths, higher quantum yield, longer lifetime and good photostability. Further experiments suggested that these N and S doped CQDs were very sensitive for the detection of Cu2+ and Hg2+, respectively.
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