期刊
JOURNAL OF MATERIALS CHEMISTRY A
卷 2, 期 12, 页码 4384-4390出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c3ta14304j
关键词
-
资金
- NSFC [21175118, 21275130]
- Colleges in Zhejiang province to the young academic leaders of academic climbing project [pd2013055]
In this report, well-dispersed porous Pt-Pd nanodendrites (Pt-Pd NDs) were synthesized at high yield by a simple, one-pot, wet chemical method without using any seed, template, or toxic organic solvent. Poly(vinylpyrrolidone) (PVP) and urea were employed as the co-stabilizing and co-structure-directing agents. It was found that the reaction temperature, the amount of PVP and urea, the Pt/Pd molar ratio, and the pH value of the reaction media greatly affected the size and shape of the Pt-Pd product. The as-prepared Pt-Pd nanocrystals had a larger active surface area, superior catalytic activity, and better stability for the electrooxidation of methanol and ethylene glycol (EG), compared with the commercial Pt-black and Pd-black catalysts.
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