期刊
JOURNAL OF MATERIALS CHEMISTRY A
卷 2, 期 18, 页码 6432-6438出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c3ta15254e
关键词
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资金
- Australian Research Council [DP0986398]
- University of New South Wales [PS26752, PS35135]
Ion exchange (IE) has been used to prepare Cu/TiO2 for photocatalytic hydrogen generation. The IE Cu/ TiO2 particles comprised a mixture of large and fine copper/copper oxide deposits which were well dispersed across the TiO2 surface. Hydrogen generation photoactivity by the IE Cu/TiO2 was similar to 44% greater than the activity displayed by Cu/TiO2 prepared via wet impregnation (WI) at a similar copper loading. Temperature programmed reduction studies indicated the IE Cu/TiO2 possessed a greater portion of highly dispersed fine copper deposits than the WI Cu/TiO2 which may account for the higher photoactivity. The hydrogen generation activity of IE Cu/TiO2 was maintained over three 5 h reaction cycles.
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