4.6 Article

Ultrathin S-doped MoSe2 nanosheets for efficient hydrogen evolution

期刊

JOURNAL OF MATERIALS CHEMISTRY A
卷 2, 期 16, 页码 5597-5601

出版社

ROYAL SOC CHEMISTRY
DOI: 10.1039/c4ta00458b

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资金

  1. MOE AcRF Tier 2 [MOE2013-T2-1-034]
  2. AcRF Tier 1 [RG 61/12, RGT18/13, RG 2/13]
  3. A*STAR SERC [1021700144]
  4. Singapore MPA [23/04.15.03]
  5. Start-Up Grant in Singapore [M4080865.070.706022]
  6. Singapore National Research Foundation under the Campus for Research Excellence And Technological Enterprise (CREATE) programme: Emobility in Megacities

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We report the synthesis of ultrathin S-doped MoSe2 nanosheets demonstrating enhanced HER catalysis with a low onset overpotential of 90 mV and a Tafel slope of 58 mV per decade. We attribute the improved catalytic effects to the proliferation of unsaturated HER active sites in MoSe2 resulting from S-doping.

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