期刊
JOURNAL OF MATERIALS CHEMISTRY A
卷 2, 期 5, 页码 1294-1301出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c3ta13687f
关键词
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资金
- National Science Foundation of China (NSFC) [21271010]
- Natural Science Foundation of Anhui Province [KJ2008B172, KJ2010ZD07]
In this study, we have demonstrated a Z-scheme photocatalytic system using Ag@AgCl encapsulated with graphene oxide (GO) (AEGO) composites, where GO and AgCl act as a highly activated photocatalyst, and metallic Ag shuttles photogenerated electrons from the excited GO and AgCl under visible light irradiation. The electron-hole pairs of the low energy level could be recombined in space by metallic Ag as a solid-state electron mediator, the remaining electron-hole pairs of the high energy level are for two photochemical reactions that operate in parallel. The Z-scheme photocatalytic system from the AEGO composite displays a much higher photocatalytic activity than Ag@AgCl-reduced graphene oxide (RGO) with the same quantitative graphene loading (15 wt%) for the degradation of methylene blue (MB). This work may provide a guide to the design of photocatalysts by the use of GO directly.
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