4.6 Article

Environment-friendly facile synthesis of Pt nanoparticles supported on polydopamine modified carbon materials

期刊

JOURNAL OF MATERIALS CHEMISTRY A
卷 1, 期 12, 页码 3945-3953

出版社

ROYAL SOC CHEMISTRY
DOI: 10.1039/c3ta00527e

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资金

  1. National Natural Science Foundation of China [21065006, 21163014]
  2. Program for New Century Excellent Talents in University [NCET-11-1002]
  3. Program for Young Scientists of Jiangxi Province [20112BCB23001]

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Pt-based catalysts are widely used in fuel cells and sensors for their exceptional electrocatalytic activity. Among the different methods for producing Pt-based catalysts, chemical reduction is favorable, due to its scalability in volume production and versatility in realizing abundant chemical functionalization. In this paper, an environment-friendly method for the facile synthesis of Pt nanoparticles supported on polydopamine (Pdop) modified carbon materials (multiwalled carbon nanotubes, carbon nanospheres and Vulcan XC-72 carbon black) is reported. Since Pdop is employed as the reductant and crosslinking agent, no reducing agents, surfactants, organic solvents, etc., are needed. The Pt-based catalysts produced using this method have a unique electrocatalytic activity toward methanol oxidation. This environmentally friendly method is promising for the synthesis of high performance catalysts for fuel cells, gas phase catalysis, and sensors.

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