期刊
IEEE JOURNAL OF PHOTOVOLTAICS
卷 4, 期 1, 页码 244-252出版社
IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC
DOI: 10.1109/JPHOTOV.2013.2289321
关键词
Hot carrier solar cell (HCSC); quantum well (QW)
In a hot carrier solar cell, the steady-state carrier population is hot relative to the surrounding lattice. This requires an absorber material which restricts carrier-phonon interaction and, therefore, reduces entropic loss during thermalization. The limiting efficiency of these devices approaches 85%: the Carnot limit for a solar energy collector. A spectroscopic analysis of GaAsP/InGaAs quantum well structures shows that carrier cooling in single quantum well samples is dominated by the rate of radiative recombination, leading to unprecedented carrier cooling lifetime (tau = 5.8 +/- 0.1 ns). This exceptional lifetime arises due to state saturation, frustrating the carrier scattering processes. A steady-state carrier population temperature >100 K above the lattice temperature is measured under illumination equivalent to 10 000 Suns. We calculate the projected efficiency >40% for a device with these characteristics, amounting to a 3% efficiency enhancement over equivalent single-junction devices.
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