期刊
ENERGY TECHNOLOGY
卷 4, 期 3, 页码 375-379出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/ente.201500296
关键词
metal alloys; molecular modeling; Seebeck coefficients; thermoelectrics; thin films
资金
- Leading Foreign Research Institute Recruitment Program through National Research Foundation of Korea - Ministry of Science, the ICT, and Future Planning (MSIP) [2011-0031643]
- Global Development Research Center
- Korea Institute for the Advancement of Technology (KIAT) - Ministry of Trade, Industry Energy (MOTIE) [N0000590]
- Thailand Research Fund (TRF) through Royal Golden Jubilee (RGJ) Ph.D. Program [PHD/0126/2556]
Thermoelectric performances are usually enhanced by minimizing the thermal conductivity of materials, either by introducing superlattice structures or nanostructuring. Here, a new approach to performance enhancement, based on Seebeck coefficient improvement, is presented for Ge2Sb2Te5 thin films. The electron temperature was controlled by using pulsed direct current (DC) plasma power, and the resulting structural disorder of the cubic crystalline phase enhanced the Seebeck coefficients, as supported by molecular orbital calculations. Our results demonstrate a room-temperature Seebeck coefficient of 190.8VK(-1) for 200nm films deposited on glass.
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