期刊
RSC ADVANCES
卷 4, 期 13, 页码 6730-6737出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c3ra47266c
关键词
-
资金
- Laboratory Directed Research and Development Program of Oak Ridge National Laboratory
- Office of Basic Energy Sciences, DOE
We report novel electrode architectures for high capacity multivalent conversion compounds such as iron (II and III) fluoride. The material and electrode design approach addresses the intrinsically poor transport and diffusion kinetics associated with ionic solids such as iron fluorides and significantly improves their electrochemical and cycle life performance. A comparison is made between the performances of 3D electrode architecture versus the slurry coated fluoride electrodes. Detailed microstructural analysis and mechanistic scenarios are discussed that would enable development of practical high energy density conversion based electrodes for energy storage application.
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