期刊
RSC ADVANCES
卷 4, 期 97, 页码 54434-54440出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c4ra09251a
关键词
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资金
- National Instrumentation Program (NIP) of the Ministry of Science and Technology of China [2011YQ03012408]
- National Natural Science Foundation of China NSFC [21373096, 21073073, 91027010]
- Innovation Program of the State Key Laboratory of Supramolecular Structure and Materials
We report a method for fabricating a highly sensitive, microfluidic surface-enhanced Raman scattering (SERS) chip with highly ordered Ag nanodot arrays as the enhancement substrate for the detection of multiplexed low-concentration analytes. The microfluidic SERS chip features a highly-ordered Ag nanodot array on quartz slides fabricated by depositing Ag with an ultrathin anodic aluminium oxide (AAO) film as template and a channel-patterned polydimethylsiloxane (PDMS) cover on top, allowing a tremendous enhancement of electromagnetic field in the proximity of the chip surface because of the localized surface plasmon resonance (LSPR) of the Ag nanodots. Via the utilization of a self-built SERS microspectrometer with an inverted configuration, the multiplexed SERS signals of low concentration adenine and thiram can be readily detected with a detection limit down to 5.0 x 10(-7) M. This detection system that we developed is flexible and has potential for real commercialization.
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