期刊
ACS PHOTONICS
卷 2, 期 8, 页码 1217-1223出版社
AMER CHEMICAL SOC
DOI: 10.1021/acsphotonics.5b00308
关键词
gold nanodisks; retardation effects; localized surface plasmon resonance; photoluminescence; oblique incidence
类别
资金
- Singapore Ministry of Education Academic Research Fund [MOE2012-T2-2-124, MOE2011-T3-1-005]
- Natural Science Foundation of China [61205042]
- Natural Science Foundation of Jiangsu Province in China [BK20141393]
- Zijin Intelligent Program of NUST [2013_zj_010203_16]
- Agency for Science, Technology and Research (A*STAR) [0926030138]
- SERC [092154099]
- National Research Foundation [NRF-CRP 8-2011-07]
Localized surface plasmon resonance (LSPR) on gold nanoparticles and nanostructures shows its capability to modulate the spontaneous emission rate for photoluminescence. However, beyond the quasi-static limit with oblique incidence conditions, probing a retardation-based plasmonic resonant state excited by the horizontal incident wave-vector component has not been reported yet in the plasmon-mediated photoluminescence of gold nanostructures. In this paper, we investigated the photoluminescence of individual and coupled gold nanodisks with increasing size, and the peaks in the size-dependent photoluminescence spectra are shown to originate from the preferential excitation of vertical (LSPR) and horizontal (retardation-based) plasmonic resonant states. We have also proposed a three-step model to well describe the contribution of vertical and horizontal plasmonic resonant states in the photoluminescence of gold nanodisks. Our study makes a new contribution to the understanding of photoluminescence from gold nanostructures, and it paves the way toward the applications of plasmon-mediated luminescence and biological studies.
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