期刊
RSC ADVANCES
卷 3, 期 34, 页码 14807-14813出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c3ra00124e
关键词
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资金
- National Natural Science Foundation of China [21207053]
- Natural Science Foundation of Jiangsu Province [BK2011460]
- Specialized Research Fund for the Doctoral Program of Higher Education [20113227110019]
- China Postdoctoral Science Foundation [2011M500861, 2012M511219, 2011M500869]
- program for Postgraduate Research Innovation in University of Jiangsu University [CXLX12_0634, CXZZ13_0693]
Transition metal ions have been immobilized on TiO2/fly-ash cenospheres (TiO2/FACs) with poly-o-phenylenediamine (OPD). The as-prepared ion imprinting photocatalyst (M-POPD/TiO2/FACs) has been characterized by SEM, XRD, FT-IR, UV-vis DRS and ICP-AES. The results demonstrated that the polymer and mental ions existed in the M-POPD/TiO2/FACs. The photocatalytic activity of M-POPD/TiO2/FACs was studied by the degradation of tetracycline, oxytetracycline, ciprofloxacin, tetracycline hydrochloride and chloromycetin in simulated wastewater under visible light irradiation. The results showed that the M-POPD/TiO2/FACs could effectively increase the separation rate of photoelectrons and holes in the cycling system and improve the photocatalytic activity for the degradation of antibiotics in solution. Experimental data showed that the as-prepared M-POPD/TiO2/FACs were more suitable for degradation of tetracycline (5 mg L-1), and the photodegradation rate could reach 71.7%. In addition, possible formation and photocatalytic mechanisms were proposed.
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