3.8 Article

Strong localization effect and carrier relaxation dynamics in self-assembled InGaN quantum dots emitting in the green

期刊

NANOSCALE RESEARCH LETTERS
卷 10, 期 -, 页码 -

出版社

SPRINGER
DOI: 10.1186/s11671-015-0772-z

关键词

InGaN; Quantum dots; Localization effect; Carrier relaxation dynamics

资金

  1. National Natural Science Foundation of China [61274052, 61106044, 11474235]
  2. Doctoral Program Foundation of Institutions of Higher Education of China [20110121110029]
  3. Fundamental Research Funds for the Central Universities [2013121024]
  4. Key Lab of Nanodevices and Nanoapplications, Suzhou Institute of Nano-Tech and Nano-Bionics of Chinese Academy of Sciences [14ZS02]

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Strong localization effect in self-assembled InGaN quantum dots (QDs) grown by metalorganic chemical vapor deposition has been evidenced by temperature-dependent photoluminescence (PL) at different excitation power. The integrated emission intensity increases gradually in the range from 30 to 160 K and then decreases with a further increase in temperature at high excitation intensity, while this phenomenon disappeared at low excitation intensity. Under high excitation, about 40% emission enhancement at 160 K compared to that at low temperature, as well as a higher internal quantum efficiency (IQE) of 41.1%, was observed. A strong localization model is proposed to describe the possible processes of carrier transport, relaxation, and recombination. Using this model, the evolution of excitation-power-dependent emission intensity, shift of peak energy, and linewidth variation with elevating temperature is well explained. Finally, two-component decays of time-resolved PL (TRPL) with various excitation intensities are observed and analyzed with the biexponential model, which enables us to further understand the carrier relaxation dynamics in the InGaN QDs.

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