期刊
ADVANCED ENERGY MATERIALS
卷 8, 期 27, 页码 -出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/aenm.201801396
关键词
electrocatalysts; flow systems; metal-air batteries; nanostructured materials; surface chemistry
类别
资金
- Joint Funds of National Natural Science Foundation of China and Guangdong Province [U1601216]
- National Natural Science Foundation of China [51602216, 51472178]
- Tianjin Natural Science Foundation [17JCQNJC02100]
- Shen-zhen Science and Technology Foundation [JCYJ20170307145703486]
- Australian Research Council (ARC) through Discovery Early Career Researcher Award [DE150101306]
- Australian Research Council (ARC) through Linkage Project [LP160100927]
As an emerging battery technology, metal-air flow batteries inherit the advantageous features of the unique structural design of conventional redox flow batteries and the high energy density of metal-air batteries, thus showing great potential as efficient electrochemical systems for large-scale electrical energy storage. This review summarizes the operating principles and recent progress of metal-air flow batteries from a materials and chemistry perspective, with particular emphasis on the latest advanced materials design and cell configuration engineering, which the authors divide into three categories based on the anode species: vanadium-air, zinc-air, and lithium-air flow batteries. Since some of the capabilities developed for metal-air static batteries can be leveraged for next-generation flow systems, classical works on conventional metal-air batteries are selected and compared with the metal-air flow systems, highlighting the prominent advantages of the latter in achieving high energy capacity and long cycle performance. At the end, a general perspective on current challenges/opportunities and future research directions to promote the commercial application of the metal-air flow battery technology is provided. The aim is to provide a comprehensive overview and to set up a road map for guiding development from conventional static to advanced flow technologies of metal-air batteries.
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