期刊
ADVANCED ENERGY MATERIALS
卷 3, 期 1, 页码 113-119出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/aenm.201200209
关键词
amorphized iron fluoride; high-capacity cathodes; porous microspheres; lithium batteries; ionic liquids; open frameworks
An FeF3 cathode with very high reversible capacity, exceeding 200 mAh g-1, is achieved by amorphizing of FeF3. The amorphization is achieved by densifying the open structure phase along with the removal of channel H2O at 0 degrees C in BmimBF4. This process is accompanied by a voltage increase of 200 mV. The generation of a hierarchical electron/ion wiring network, enabled by the interaction of ionic liquid with carbon nanotube and FeF3 surfaces, significantly improves the reversibility.
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