期刊
ACS CATALYSIS
卷 5, 期 2, 页码 627-630出版社
AMER CHEMICAL SOC
DOI: 10.1021/cs501510e
关键词
water splitting; copper; electrocatalysis; water oxidation; thin film
资金
- National Basic Research Program of China [2014CB239402]
- National Natural Science Foundation of China [21476043, 21120102036, 21361130020]
- Natural Science Foundation of Liaoning Province, China [2014020010]
- Fundamental Research Funds for the Central Universities [DUT14YQ104]
- Swedish Energy Agency
- K&A Wallenberg Foundation
A robust water oxidation catalyst based on copper oxide was prepared by facile electrodeposition of Cu2+ from borate buffer solution under near neutral conditions. The Cu-B-i thin film exhibits high activity and long-term stability in Cu2+-free pH 9 borate buffer. A steady current density of 1.2 mA/cm(2) was sustained for at least 10 h at 1.3 V versus NHE without iR compensation, which sets a new benchmark for copper-based OEC.
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