期刊
JOURNAL OF MATERIALS CHEMISTRY C
卷 3, 期 37, 页码 9726-9733出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c5tc02017d
关键词
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资金
- National Natural Science Foundation of China [112064038, 61275153, 61320206014]
- European Regional Development Fund-FESR of POR Campania - Call Innovation Window
- K. C. Wong Magna Foundation of Ningbo University, China
Well-shaped Ag@Au hexagonal nanorings (Ag@Au HNRs) were successfully synthesized with the assistance of Ag hexagonal nanoplates as structure-directing templates in a galvanic replacement route, and their optical characteristics were studied in detail. During the synthetic process, the morphology of the Ag@Au HNRs was found to be strongly depended on the dosage of HAuCl4 added into the template solution. Both the experimental and calculated absorption spectra showed that the red-shift of localized surface plasmon resonance (LSPR) peaks of the Ag@Au HNRs obeyed a modified Lorentz function with increasing dosage of HAuCl4 solution, which was also explained by the plasmon hybridization of the Ag@Au HNRs. Moreover, the surface-enhanced Raman scattering (SERS) characteristics of Ag@Au HNRs were investigated by using 4-mercaptobenzoic acid (4MBA) as a Raman reporter molecule. And the as-prepared Ag@Au HNRs exhibit excellent SERS performances with an enhancement factor similar to 10(6), especially for the Ag@Au HNR prepared at 160 mu l HAuCl4 solution due to its strongest plasmon electric-field enhancement. It reveals that the as-synthesized Ag@Au HNRs possess great potential for the application in ultrasensitive biosensors.
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