期刊
CHEMICAL SCIENCE
卷 5, 期 5, 页码 2052-2056出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c4sc00081a
关键词
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资金
- Aarhus University
- Carlsberg Foundation
- CONACYT (Mexico)
The [4+2]-cycloaddition reaction of 3-olefinic oxindoles with a tetraenamine intermediate is presented. In the reaction, a novel class of highly functionalized spirocyclic cyclohexanes with four stereocenters is formed in high yield and excellent stereoselectivity. Mechanistic investigations and calculations point to a stepwise mechanism involving tetraenamine intermediates. Furthermore, several transformations are presented.
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