期刊
CHEMICAL SCIENCE
卷 4, 期 9, 页码 3573-3577出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c3sc51336j
关键词
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资金
- European Research Council
- Cambridge Overseas Trust
- Australian Research Council
The synthesis of stable bicontinuous hierarchically porous metal-organic frameworks (MOFs) is described. Two functional block co-oligomer templates were used independently, i.e. poly(styrene)-block-poly(4-vinylpyridine) and poly(styrene)-block-poly(acrylic acid). Two prototypical MOFs, ZIF-8 and HKUST-1, were selected to demonstrate our approach. The resulting materials resemble the microstructures of bicontinuous silica aerogels. They exhibit interconnected porosities throughout the micro-, meso- and macro-porous regions, as shown by electron microscopy and pore size distribution analyses.
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