期刊
CHEMICAL SCIENCE
卷 3, 期 4, 页码 1095-1099出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c2sc00943a
关键词
-
资金
- NSF CAREER [CHE-0548003]
- University of Florida
Synthetic access to discrete multifunctionalized molecules remains a challenge but is critical for continued advances in materials science, catalysis, and chemical biology. Here, the aminolysis of electronically coupled lactones is introduced as an approach to achieve molecular multifunctionalization efficiently, under mild conditions, and without protecting groups or by-products. The one-pot sequential aminolysis of benzotrifuranone, a C-3h-symmetric trilactone, to produce a trifunctionalized target in similar to 85% yield over one day is highlighted.
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