期刊
CHEMICAL SCIENCE
卷 3, 期 1, 页码 205-208出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c1sc00517k
关键词
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资金
- National Basic Research Program of China (973 Program) [2009CB825300]
- NSFC [20821002, 20923005, 21025209]
- Chinese Academy of Sciences
Asymmetric dearomatization of pyrroles has been accomplished by using Ir-catalyzed intramolecular asymmetric allylic alkylation reactions. Reactions of allylic carbonate tethered pyrroles in the presence of [Ir(cod)Cl](2) and a BINOL-derived phosphoramidite ligand lead to efficient generation of spiro-2H-pyrrole derivatives with up to 96% ee.
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