期刊
CHEMICAL SCIENCE
卷 3, 期 6, 页码 1879-1882出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c2sc20096a
关键词
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资金
- NSFC [20972101, 21021001, 21125206]
- National Basic Research Program of China (973 Program) [2010CB833300]
An asymmetric inverse-electron-demand Diels-Alder reaction of chromone-fused dienes and beta, beta-disubstituted alpha,beta-unsaturated aldehydes has been developed via dienamine catalysis. Different domino or sequential transformations could be carried out for electron-deficient dienes with variously substituted patterns, allowing for the efficient construction of caged or fused tetrahydroxanthones with high molecular complexity and skeletal diversity in excellent diastereo- and enantioselectivities.
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