期刊
CHEMICAL SCIENCE
卷 2, 期 2, 页码 312-315出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c0sc00367k
关键词
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资金
- GSK
- EPSRC
- Marie Curie Foundation
- Royal Society for University
- Philip Patricia Brown
Pd(II)-catalyzed C-H bond functionalizations that proceed under ambient conditions are a pivotal part of the future of chemical synthesis. Herein, an amine directed Pd(II)-catalyzed C-H bond functionalization strategy is described that generates a diversity of molecular frameworks via C-H carbonylation, C-H arylation and C-H amination. The new reactions work for a variety of substrates and are tolerant of delicate stereogenic centres and functionality. Furthermore, the new reactions can be sequenced to generate complex architectures from simple building blocks via iterative Pd(II)-catalyzed C-H bond functionalization.
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