期刊
CHEMICAL SCIENCE
卷 2, 期 8, 页码 1519-1522出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c1sc00083g
关键词
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资金
- NSFC [20732006, 20821002, 21025209, 21002111]
- MOST [2010CB833300]
- CNIBR
Desymmetrization of cyclohexadienones via aza-Michael reaction catalyzed by cinchonine derived thiourea has been realized to afford a series of highly enantioenriched pyrrolidine and morpholine derivatives in excellent yields and ees. With this newly established methodology, asymmetric total synthesis of (-)-Mesembrine in high enantiomeric excess (98% ee) was accomplished.
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