期刊
CHEMICAL SCIENCE
卷 2, 期 7, 页码 1401-1406出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c1sc00199j
关键词
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资金
- National 973 Program [2007CB936702, 2011CBA00702]
- National Science Foundation of China [50973105]
- CAS [KGCX2-YW-326]
The iodide/triiodide redox shuttle is an unparalleled option in making efficient dye-sensitized solar cells (DSCs) but also presents some prominent constraints on the development of new photosensitizers, semiconductors and counter electrodes. In this paper, a cobalt electrolyte has been identified to offer an advantageous impact of pi-conjugation extension in push-pull organic dyes, upon the interfacial charge recombination kinetics and thus the open-circuit photovoltage of DSCs, in sharp contrast with the conventional iodine congener. The usage of a solely visible-light-absorption dye has generated a DSC free of corrosive iodine, exhibiting an impressive overall power conversion efficiency of 8.0% at the 100 mW cm(-2) AM1.5G conditions.
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