期刊
JOURNAL OF MATERIALS CHEMISTRY A
卷 3, 期 4, 页码 1504-1510出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c4ta05573j
关键词
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资金
- National Natural Science Foundation of China [21376001]
- Excellent Young Scholars Research Fund of Beijing Institute of Technology [2013YR1013]
A three-dimensional (3D) graphene-Co3O4 electrode was prepared by a two-step method in which graphene was initially deposited on a Ni foam with Co3O4 then grown on the resulting graphene structure. Cross-linked Co3O4 nanosheets with an open pore structure were fully and vertically distributed throughout the graphene skeleton. The free-standing and binder-free monolithic electrode was used directly as a cathode in a Li-O-2 battery. This composite structure exhibited enhanced performance with a specific capacity of 2453 mA h g(-1) at 0.1 mA cm(-1) and 62 stable cycles with 583 mA h g(-1) (1000 mA h g(carbon)(-1)). The excellent electrochemical performance is associated with the unique architecture and superior catalytic activity of the 3D electrode.
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