期刊
TOPICS IN CATALYSIS
卷 53, 期 15-18, 页码 1132-1137出版社
SPRINGER/PLENUM PUBLISHERS
DOI: 10.1007/s11244-010-9546-0
关键词
Iridium; Palladium; Bimetallic catalysts; Benzonitrile; Hydrogenation
资金
- National Action Council for Minorities in Engineering (NACME), Inc.
- NSF
- SEAGEP
The kinetics of liquid-phase hydrogenation of benzonitrile have been examined alumina supported Ir, Pd and Ir-Pd catalysts. Benzonitrile disappearance TOF is 10-fold higher for Pd catalyst than it is for Ir catalyst. Benzylamine is produced preferentially over Pd, whereas dibenzylamine is produced principally over Ir. Non-monotonic activity and selectivity relationships with bimetallic composition are obtained.
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