期刊
TETRAHEDRON LETTERS
卷 53, 期 12, 页码 1485-1489出版社
PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/j.tetlet.2012.01.040
关键词
Hydroarylation; Heterogeneous catalyst; Nanoporous; Catalysis; FeAl-KIT-5
资金
- Ministry of Education, Culture, Sports, Science, and Technology (MEXT)
- World Premier International Research Center (WPI) Initiative on Materials Nanoarchitectonics, MEXT, Japan
A novel bimetallic nanoporous FeAl-KIT-5 catalyst with a cage type porous structure and a high surface area has been prepared for the hydroarylation of styrene and arylacetylenes to afford 1,1-diarylalkanes and 1,1-diarylalkenes, respectively. The catalyst was found to be highly active, and selective, affording a high yield of substituted alkanes and alkenes. The catalyst also showed much higher activity as compared to those of other nanoporous catalysts such as AISBA-15, AIKIT-5, and FeKIT-5, and can be reused several times without much loss of its activity. Crown Copyright (C) 2012 Published by Elsevier Ltd. All rights reserved.
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