期刊
TETRAHEDRON LETTERS
卷 53, 期 21, 页码 2588-2591出版社
PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/j.tetlet.2012.03.021
关键词
Daphniphyllum oldhami; Daphniphyllum alkaloid; Daphnioldhamine A; Transannular effect
资金
- Chinese National Natural Science Foundation [30830114, 31100259, 30800092]
- Chinese Ministry of Science and Technology [2009CB522300, 2009CB940900]
- Young Academic and Technical Leader Raising Foundation of Yunnan Province [2009CI072]
Daphnioldhamine A, the first Daphniphyllum alkaloid with transannular effect, easily tautomerized under acidic or alkaline conditions, was isolated from the fruits of Daphniphyllum oldhami. The structure was elucidated by spectroscopic and computational approaches and chemical transformation. A plausible biosynthetic pathway of daphnioldhamine A was also proposed. (C) 2012 Elsevier Ltd. All rights reserved.
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